Journal
ADVANCED FUNCTIONAL MATERIALS
Volume 26, Issue 46, Pages 8478-8486Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adfm.201603734
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Funding
- State Key Laboratory of Pulsed Power Laser Technology of China in Electronic Engineering Institute (Hefei) [SKL 2015 KF04]
- National Natural Science Foundation of China [61076040, U1632151]
- Specialized Research Fund for the Doctoral Program of Higher Education of China [2012011111006]
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Cesium lead halide quantum dots (QDs) have tunable photoluminescence that is capable of covering the entire visible spectrum and have high quantum yields, which make them a new fluorescent materials for various applications. Here, the synthesis of CsPbX3 (X = Cl, Br, I, or mixed Cl/Br and Br/I) QDs by direct ion reactions in ether solvents is reported, and for the first time the synergetic effects of solvent polarity and reaction temperature on the nucleation and growth of QDs are demonstrated. The use of solvent with a low polarity enables controlled growth of QDs, which facilitates the synthesis of high-quality CsPbX3 QDs with broadly tunable luminescence, narrow emission width, and high quantum yield. A QD white LED (WLED) is demonstrated by coating the highly fluorescent green-emissive CsPbBr3 QDs together with red phosphors on a blue InGaN chip, which presents excellent warm white light emission with a high rendering index of 93.2 and color temperature of 5447 K, suggesting the potential applications of highly fluorescent cesium lead halide perovskite QDs as an alternative color converter in the fabrication of WLEDs.
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