Journal
SCIENCE ADVANCES
Volume 5, Issue 1, Pages -Publisher
AMER ASSOC ADVANCEMENT SCIENCE
DOI: 10.1126/sciadv.aav0363
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Funding
- National Natural Science Foundation of China [51722202, 91622125, 51572023, 11574003]
- Natural Science Foundations of Beijing [2172036]
- National Science Foundation [DMR-1608218]
- French National Agency for Research [ANR-16-CE08-0003-01]
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Solid-state phosphor-converted white light-emitting diodes (pc-WLEDs) are currently revolutionizing the lighting industry. To advance the technology, phosphors with high efficiency, tunable photoluminescence, and high thermal stability are required. Here, we demonstrate that a simple lithium incorporation in NaAlSiO4: Eu system enables the simultaneous fulfillment of the three criteria. The Li substitution at Al sites beside Na sites in NaAlSiO4: Eu leads to an enhanced emission intensity/efficiency owing to an effective Eu3+ to Eu2+ reduction, an emission color tuning from yellow to green by tuning the occupation of different Eu sites, and an improvement of luminescence thermal stability as a result of the interplay with Li-related defects. A pc-WLED using the Li-codoped NaAlSiO4: Eu as a green component exhibits improved performance. The phosphors with multiple activator sites can facilitate the positive synergistic effect on luminescence properties.
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