Journal
SCIENCE OF THE TOTAL ENVIRONMENT
Volume 648, Issue -, Pages 902-915Publisher
ELSEVIER
DOI: 10.1016/j.scitotenv.2018.08.181
Keywords
Air pollution; Meteorological factors; Spatial econometric model; China
Categories
Funding
- National Natural Science Foundation of China [91744205, 21777025, 21577022, 21177026]
- National Key R&D Program of China [2016YFC0202700]
- International Cooperation Project of Shanghai Municipal Government [15520711200]
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With rapid economic development and urbanization, China has suffered from severe and persistent air pollution during the past years. In the work, the hourly data of PM2.5, PM10, SO2, NO2, CO, and O-3 in all of the prefecturelevel cities (336 cities) during 2015-2016were collected to uncover the spatiotemporal variations and influential factors of these pollutants in China. The average concentrations of PM2.5, PM10, SO2, NO2, and CO decreased by 19.32%, 15.34%, 29.30%, 9.39%, and 8.00% from 2015 to 2016, suggesting the effects of efficient control measurements during this period. On the contrary, the O-3 concentration increased by 4.20% during the same period, which mainly owed to high volatile organic compounds (VOCs) loading. The concentrations of PM2.5, PM10, SO2, CO and NO2 showed the highest and the lowest ones in winter and summer, respectively. However, the O-3 concentration peaked in summer, followed by ones in spring and autumn, and presented the lowest one in winter. All of the pollutants exhibited significantly weekly and diurnal cycle in China. PM2.5, PM10, SO2, CO and NO2 presented the higher concentrations onweekdays than those atweekends, all ofwhich showed the bimodal pattern with two peaks at late night (21: 00-22: 00) and inmorning (9: 00-10: 00), respectively. However, the O-3 concentration exhibited the highest value around 15: 00. The statistical analysis suggested that the PM2.5, PM10, and SO2 concentrations were significantly associated with precipitation (Prec), atmosphere temperature (T), and wind speed (WS). The CO and NO2 concentrations displayed the significant relationship with T, while the O-3 concentration was closely linked to the sunshine duration (Tsun) and relative humidity (RH). T and WS were major factors affecting the accumulation of PM and gaseous pollutants at a national scale. At a spatial scale, Prec and T played the important roles on the PM distribution in Northeast China, and the effect of Prec on CO concentration decreased fromSoutheast China to Northwest China. The results shown herein provide a scientific insight into the meteorology impacts on air pollution over China. (C) 2018 Elsevier B.V. All rights reserved.
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