Journal
PHYSICAL REVIEW LETTERS
Volume 121, Issue 22, Pages -Publisher
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.121.227401
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Funding
- European Research Council [ERC-2011-AdG-290981, ERC-2016-STG-714870]
- European Union [FP7-PEOPLE-2013-CIG-618229]
- Spanish MINECO [MAT2014-53432-C5-5-R]
- Maria de Maeztu programme for Units of Excellence in RD [MDM-2014-0377]
- EPSRC
- Winton Programme for the Physics of Sustainability
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We calculate the exact many-body time dynamics of polaritonic states supported by an optical cavity filled with organic molecules. Optical, vibrational, and radiative processes are treated on an equal footing employing the time-dependent variational matrix product states algorithm. We demonstrate signatures of non-Markovian vibronic dynamics and its fingerprints in the far-field photon emission spectrum at arbitrary light-matter interaction scales, ranging from the weak to the strong coupling regimes. We analyze both the single-and many-molecule cases, showing the crucial role played by the collective motion of molecular nuclei and dark states in determining the polariton dynamics and the subsequent photon emission.
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