Journal
ORGANIC LETTERS
Volume 20, Issue 23, Pages 7433-7436Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.8b03162
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Funding
- Ministry of Education (MOE) of Singapore [R-143-000-613-112]
- A*STAR SERC [R-143-000-648-305]
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Unprecedented one-pot thiocyanofunctionalizations of terminal alkynes to deliver alkynylthiocyanates and alpha-thiocyanoketones using a silver-catalyzed procedure or under silver/gold relay catalysis is reported. These synthetically valuable organothiocyanates are accessed in high efficiency, and their derivatization into a variety of valuable sulfur-containing heterocycles and sulfides has also been demonstrated.
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