Journal
ORGANIC LETTERS
Volume 20, Issue 23, Pages 7641-7644Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.8b03378
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Funding
- National Natural Science Foundation of China [21871160, 21672121]
- Thousand Plan Youth Program of China
- Tsinghua University
- Bayer Investigator Fellow
- Fellowship of Tsinghua-Peking Centre for Life Sciences (CLS)
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A new carbene-catalyzed [4 + 2] annulation of 2H-azirine-2-carbaldehydes with ketones was developed, thus providing the 2,3-dihydro-6H-1,3-oxazin-6-one core structures with broad scope and good to excellent yields. Notably, the azolium aza-dienolates generated from the addition of NHCs to 2H-azirines are first uncovered.
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