Journal
ORGANIC LETTERS
Volume 21, Issue 1, Pages 218-222Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.8b03666
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Funding
- National Key Research and Development Program of China [2016YFA0602900]
- 1000 Youth Talents Plan
- Fundamental Research Funds for the Central Universities [2017ZD060]
- National Natural Science Foundation of China [21472052]
- Science and Technology Program of Guangzhou [201607010306]
- Science Foundation for Distinguished Young Scholars of Guangdong Province [2014A030306018]
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A cobalt-catalyzed site-selective functionalization of aniline derivatives with hexafluoroisopropanol, which enables the synthesis of a wide array of fluoroalkylated anilines, a class of highly valuable building blocks for further preparation of fluorinated functional products, is reported. The developed transformation proceeds with operational simplicity, use of earth-abundant metal catalyst, broad substrate scope, good functional group tolerance, and mild reaction conditions.
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