Journal
ACS NANO
Volume 10, Issue 8, Pages 7231-7247Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acsnano.6b03349
Keywords
graphene; polymer; three-dimensional; composites; environment; energy; sensor
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Funding
- Program for Professor of Special Appointment (Eastern Scholar) at Shanghai Institutions of Higher Learning [TP2015002]
- National Natural Foundation of China [51403099]
- U.S. National Science Foundation [DMRI508144]
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Integration of graphene with polymers to construct three-dimensional porous graphene/polymer composites (3DGPCs) has attracted considerable attention in the past few years for both fundamental studies and diverse technological applications. With the broad diversity in molecular structures of graphene and polymers via rich chemical routes, a number of 3DGPCs have been developed with unique structural, electrical, and mechanical properties, chemical tenability, and attractive functions, which greatly expands the research horizon of graphene-based composites. In particular, the properties and functions of the 3DGPCs can be readily tuned by precisely controlling the hierarchical porosity in the 3D graphene architecture as well as the intricate synergistic interactions between graphene and polymers. In this paper, we review the recent progress in 3DGPCs, including their synthetic strategies and potential applications in environmental protection, energy storage, sensors, and conducting composites. Lastly, we will conclude with a brief perspective on the challenges and future opportunities.
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