Journal
ACS APPLIED MATERIALS & INTERFACES
Volume 8, Issue 23, Pages 14521-14526Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acsami.6b02331
Keywords
MoS2; nickel; core/shell nanosheets array; synergistic effect; hydrogen evolution reaction
Funding
- National Natural Science Foundation of China [21435005, 21575137]
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Hydrogen evolution reaction (HER) in alkaline media using non-noble Metal catalysts with great efficiency represents a critical challenge in current water-alkaline and Chlor-alkali electrolyzers. Herein; we demonstrate that the MoS2@Ni core/shell nanosheets array vertically aligned on carbon. cloth (MoS2@Ni/CC) is a highly active electrocatalyst for HER. In alkaline solutions, MoS2@Ni/CC needs over potentials of 91, 118, and 196 mV to approach current densities of 10, 20, and 100 mA cm(-2), respectively, exceeding behavior of commercial Pt/C catalyst at high current densities. Additionally:, this catalyst also exhibits excellent electrocatalytic activity toward HER in neutral electrolytes. Such high hydrogen evolution activities are due to synergistic electrocatalytic,effects between MoS2 core and Ni shell.
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