4.8 Article

Very Bright and Efficient Microcavity Top-Emitting Quantum Dot Light-Emitting Diodes with Ag Electrodes

Journal

ACS APPLIED MATERIALS & INTERFACES
Volume 8, Issue 26, Pages 16768-16775

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acsami.6b03367

Keywords

quantum dot; light-emitting diodes; top-emitting structures; microcavity effect; silver electrodes

Funding

  1. Basic Research Program of Science, Technology and Innovation Commission of Shenzhen Municipality [JCYJ20140417105742713]
  2. National Natural Science Foundation of China [61405089, 11274402]
  3. Guangdong Natural Science Funds for Distinguished Young Scholars [2016A030306017]
  4. Guangdong Special Support Program for Young Talent Scholar [2014TQ01x015]
  5. Natural Science Foundation of Guangdong Province [S2012020011003]

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The microcavity effect in top-emitting quantum dot light emitting diodes (TQLEDs) is theoretically and experimentally investigated. By carefully optimizing the cavity length, the thickness of the top Ag electrode and the thickness of the capping layer, very bright and efficient TQLEDs with external quantum efficiency (EQE) of 12.S% are demonstrated. Strong dependence of luminance and efficiency on cavity length is observed, in good agreement with theoretical calculation. By setting the normal-direction resonant wavelength around the peak wavelength of the intrinsic emission, highest luminance of 112 000 cd/m(2) (at a driving voltage of 7 V) and maximum current efficiency of 27.8 cd/A are achieved, representing a 12-fold and a 2.1-fold enhancement compared to 9000 cd/m(2) and 13.2 cd/A of the conventional bottom emitting devices, respectively, whereas the highest EQE of 12.5% is obtained by setting the resonant wavelength 30 nm longer than the peak wavelength of the intrinsic emission. Benefit from the very narrow spectrum of QDs and the low absorption of silver electrodes, the potential of microcavity effect can be fully exploited in TQLEDs.

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