Journal
ACS APPLIED MATERIALS & INTERFACES
Volume 8, Issue 11, Pages 7173-7183Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acsami.6b01116
Keywords
selective sensing gas; metal functionalization; catalyst; d-band; theory
Funding
- Inha University
- SUTD-ZJU grant on chemical thermodynamics [SUTD-ZJU/RES/01/2012]
- Singapore MOE [MOE 2012-T2-1-097]
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We have fabricated multiple networked SnO2 nanowires and subsequently decorated-them with uniformly distributed metal nanoparticles (NPs). The sensing tests indicated that the Pt-, Pd-, and Au-decorated SnO2 nanowires exhibited excellent sensing behavior, specifically for C7H8, C6H6, and CO gases, respectively. We discussed the associated sensing mechanisms in regard to the selective catalytic effects of metal NPs. In addition, by means of d-band theory, we explained the catalytic capabilities of each metal and proposed design principles for exploring new catalytic metals. The present study will pave the way for further development of high-selectivity sensors.
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