4.8 Article

Suppression of Interfacial Current Fluctuation in MoTe2 Transistors with Different Dielectrics

Journal

ACS Applied Materials & Interfaces
Volume 8, Issue 29, Pages 19092-19099

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acsami.6b02085

Keywords

MoTe2 transistor; low-frequency noise; interfacial Coulomb scattering; carrier number/mobility fluctuation; h-BN gate dielectric

Funding

  1. Nano-Material Technology Development Program through National Research Foundation of Korea (NRF)
  2. Ministry of Science, ICT and Future Planning [2009-0082580, 2015069202]
  3. Institute for Basic Science, Republic of Korea [IBS-R011-D1]

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For transition metal dichalcogenides, the fluctuation of the channel current due to charged impurities is attributed to a large surface area and a thickness of a few nanometers. To investigate current variance at the interface of transistors, we obtain the low-frequency (LF) noise features of MoTe2 multilayer field-effect transistors with different dielectric environments. The LF noise properties are analyzed using the combined carrier mobility and carrier number fluctuation model which is additionally parametrized with an interfacial Coulomb-scattering parameter (a) that varies as a function of the accumulated carrier density (Nacc) and the location of the active channel layer of MoTe2. Our model shows good agreement with the current power spectral density (PSD) of MoTe2 devices from a low to high current range and indicates that the parameter a exhibits a stronger dependence on Nacc with an exponent -gamma, of -1.18 to approximately -1.64 for MoTe2 devices, compared with -0.5 for Si devices. The raised Coulomb scattering of the carriers, particularly for a low-current regime, is considered to be caused by the unique traits of layered semiconductors such as interlayer coupling and the charge distribution strongly affected by the device structure under a gate bias, which completely change the charge screening effect in MoTe2 multilayer. Comprehensive static and LF noise analyses of MoTe2 devices with our combined model reveal that a chemical-vapor deposited h-BN monolayer underneath MoTe2 channel and the Al2O3 passivation layer have a dissimilar contribution to the reduction of current fluctuation. The three-fold enhanced carrier mobility due to the h-BN is from the weakened carrier scattering at the gate dielectric interface and the additional 30% increase in carrier mobility by Al2O3 passivation is due to the reduced interface traps.

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