Journal
ACS APPLIED MATERIALS & INTERFACES
Volume 8, Issue 7, Pages 4523-4531Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acsami.5b10830
Keywords
perovskite solar cells; silver nanowires; composite metallic; top electrode; semitransparent
Funding
- Ministry of Science & Technology, Israel
- Ministry of Science & Technology, P.R. China
- China-Israel Cooperative Scientific Research Fund [2015DFG52690]
- NSFC [51561145007]
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We report herein perovskite solar cells using solution-processed silver nanowires (AgNWs) as transparent top electrode with markedly enhanced device performance, as well as stability by evaporating an ultrathin transparent Au (UTA) layer beneath the spin-coated AgNWs forming a composite transparent metallic electrode. The interlayer serves as a physical separation sandwiched in between the perovskite/hole transporting material (HTM) active layer and the halide-reactive AgNWs top-electrode to prevent undesired electrode degradation and simultaneously functions to significantly promote ohmic contact. The as-fabricated semitransparent PSCs feature a V-oc of 0.96 V, a J(sc) of 20.47 mA cm(-2), with an overall PCE of over 11% when measured with front illumination and a V-oc of 0.92 V, a J(sc) of 14.29 mA cm(-2), and an overall PCE of 7.53% with back illumination, corresponding to approximately 70% of the value under normal illumination conditions. The devices also demonstrate exceptional fabrication repeatability and air stability.
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