Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 141, Issue 1, Pages 48-52Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jacs.8b09945
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Funding
- National Nature Science Foundation of China [21672222, 21790050, 21790051]
- NSFC-DFG joint fund [21661132006]
- National key research and development project of China [2016YFA0200104]
- Chinese Academy of Science [QYZDY-SSW-SLH015]
- Strategic Priority Research Program of the Chinese Academy of Sciences [XDA09020302]
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The synthesis of graphdiyne with an ordered internal structure is highly attractive for its various scientific and application investigations. We reported herein a rational method to fabricate a graphdiyne analogue with the help of supramolecular chemistry. The introduction of pi-pi/CH-pi interactions controlled the conformations of the precursors and afforded multilayer graphdiyne analogue Ben-GDY through the wet chemical method. The in-plane periodicity of the multilayer Ben-GDY was corroborated by transmission electron microscopy and selected area electron diffraction, which showed a pattern well matched with ABC-style stacking.
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