4.5 Article

Dynamics of the magnetoelastic phase transition and adiabatic temperature change in Mn1.3Fe0.7P0.5Si0.55

Journal

JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS
Volume 477, Issue -, Pages 287-291

Publisher

ELSEVIER SCIENCE BV
DOI: 10.1016/j.jmmm.2018.12.086

Keywords

Magnetic cooling; Dynamical effects; First-order transition; Fe2P; High magnetic-fields

Funding

  1. European Research Council (ERC) under the European Unions Horizon 2020 research and innovation programme [743116]
  2. DFG [SPP 1599]
  3. European Community [310748]
  4. HLD at HZDR, member of the European Magnetic Field Laboratory (EMFL)

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The adiabatic temperature change Delta T-ad of a Mn1.3Fe0.7P0.5Si0.55 Fe2P-type alloy was measured under different magnetic field-sweep rates from 0.93 Ts-1 to 2870 Ts-1. We find a field-sweep-rate independent magnetocaloric effect due to a partial alignment of magnetic moments in the paramagnetic region overlapping with the magnetocaloric effect of the first-order phase transition. Additionally, the first-order phase transition is not completed even in fields up to 20 T leading to a non-saturating behavior of Delta T-ad. Measurements in different pulsed fields reveal that the first-order phase transition cannot follow the fast field changes as previously assumed, resulting in a distinct field-dependent hysteresis in Delta T-ad.

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