Journal
JOURNAL OF ENVIRONMENTAL SCIENCES
Volume 80, Issue -, Pages 159-168Publisher
SCIENCE PRESS
DOI: 10.1016/j.jes.2018.12.008
Keywords
Ag-modified manganese oxide; Ag-Hollandite; Ozone decomposition; Co-precipitation method
Categories
Funding
- National Key R&D Program of China [2016YFC0207104, 2017YFC0211802]
- National Natural Science Foundation of China (NSFC) [21876191]
- Youth Innovation Promotion Association, Chinese Academy of Sciences [2017064]
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O-3 decomposition catalysts with excellent performance still need to be developed. In this study, Ag-modified manganese oxides (AgMnOx ) were synthesized by a simple co-precipitation method. The effect of calcination temperature on the activity of MnOx and AgMnOx catalysts was investigated. The effect of the amount of Ag addition on the activity and structure of the catalysts was further studied by activity testing and characterization by a variety of techniques. The activity of 8%AgMnOx for ozone decomposition was significantly enhanced due to the formation of the Ag1.8Mn8O16 structure, indicating that this phase has excellent performance for ozone decomposition. The weight content of Ag1.8Mn8O16 in the 8%AgMnOx catalyst was only about 33.76%, which further indicates the excellent performance of the Ag1.8Mn8O16 phase for ozone decomposition. The H-2 temperature programmed reduction (H-2 -TPR) results indicated that the reducibility of the catalysts increased due to the formation of the Ag1.8Mn8O16 structure. This study provides guidance for a follow-up study on Ag-modified manganese oxide catalysts for ozone decomposition. (C) 2018 The Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences. Published by Elsevier B.V.
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