Journal
INORGANIC CHEMISTRY
Volume 57, Issue 22, Pages 14018-14022Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.inorgchem.8b02031
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Funding
- National Natural Science Foundation of China [21601047, 21501094]
- Natural Science Fund of Jiangsu Province [BK20150798]
- Fundamental Research Funds for the Central Universities [2018B17614]
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In this work, we employed a new tetrazolyl-functionalized ligand, 5-(1H-tetrazole-5-yl)-1,3-bis(3,5-dicarboxylpheny1)-benzene (H5TBDPB), and successfully obtained an example of incorporating free tetrazolyl groups in transition-metal-based MOFs based upon an ideal MOF platform. With a BET surface area of 2070 m(2) g(-1), this new tetrazolyl-decorated MOF [Cu-6(TBDPB)(3)(H2O)center dot 9DMF center dot 15H(2)O (HHU-5, HHU for Hohai University) exhibits a high CO2 adsorption capacity of 37.1 wt % at 1 bar and 273 K and high CO2 separation capacity toward N-2 and CH4 as well.
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