Journal
FULLERENES NANOTUBES AND CARBON NANOSTRUCTURES
Volume 26, Issue 12, Pages 804-809Publisher
TAYLOR & FRANCIS INC
DOI: 10.1080/1536383X.2018.1502176
Keywords
Carbon nanotubes; ethylene; hydrogenation; carbocatalyst; metal-free catalyst
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Funding
- program New functional compounds and materials of chemical production of the National Academy of Sciences of Ukraine [5-18]
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This work shows, for the first time, that the multi-walled carbon nanotubes (MWCNTs) exhibit the catalytic activity in the ethylene hydrogenation. MWCNTs with the average diameter of 35 nm were prepared by CVD from ethylene as a carbon source at 700 degrees C. TEM, SEM, and XRD indicate that MWCNTs are characterized by a sufficiently high defectiveness. FTIR highlights that the catalytic process occurs in the presence of the hydroxyl and carbonyl surface groups. We demonstrate the high catalytic stability of MWCNTs at temperatures up to 400 degrees C.
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