Journal
EUROPEAN JOURNAL OF INORGANIC CHEMISTRY
Volume -, Issue 39, Pages 4322-4330Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/ejic.201800579
Keywords
Zinc; N; O-ligands; Aggregation-induced emission; Solution-processed white organic light-emitting diodes (WOLEDs)
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Funding
- Natural Sciences and Engineering Research Council (NSERC)
- le Fonds du Quebec pour la recherche sur la nature et les technologies (FRQNT)
- Centre for Self-Assembled Chemical Structures (CSACS)
- Centre in Green Chemistry and Catalysis (CGCC)
- Universite de Montreal (UdeM)
- CREATE program (Novel Chiral Materials: An International Effort in Research and Education)
- [RGPIN-2015-05485]
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The synthesis, characterization, photophysical and redox properties of a dinuclear complex Zn-2(AMOX)(4) (AMOX = 4-bromo-N,N-diphenylbenzamidinate N-oxide) are highlighted. This compound is a first example of a novel class of aggregation-induced emission (AIE) materials. Noticeably, solution-processed white-green organic light-emitting diodes were fabricated using this complex as dopant in a co-host matrix in the emissive layer. A luminance efficiency and power efficiency as high as 1.12 cd/A and 0.30 lm/W were obtained, respectively. The characteristics of this complex: high solubility, thermal stability, AIE behaviour, ease of synthesis, tunability options, and low-cost, reveal altogether great potential for the development of this new family of compounds as materials for applications in optoelectronic devices.
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