Journal
CHINESE JOURNAL OF CHEMISTRY
Volume 36, Issue 12, Pages 1187-1190Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/cjoc.201800369
Keywords
asymmetric catalysis; C-H functionalization; 2H-chromene; aldehyde; oxidation; synthetic method
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Funding
- National Natural Science Foundation of China [21722204, 21472112]
- Fok Ying Tung Education Foundation [151035]
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The first catalytic asymmetric cross-dehydrogenative coupling of 2H-chromenes with aldehydes using o-chloranil (3,4,5,6-tetrachloro-1,2- benzoquinone) as an oxidant has been described. The organocatalytic process is tolerated with a broad range of structurally and electronically varied 2H-chromenes and aldehydes with good yield and high enantiocontrol.
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