Journal
CHEMISTRY-A EUROPEAN JOURNAL
Volume 24, Issue 72, Pages 19166-19170Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/chem.201805441
Keywords
C-H activation; electrochemistry; mechanism; nickel catalysis; nickel(IV); selectivity
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Funding
- CSC
- DFG (Gottfried-Wilhelm-Leibniz award)
- Alexander-von-Humboldt foundation
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Nickel-catalyzed electrochemical C-H aminations were accomplished by chemo- and position-selective C-H activation with ample scope. Detailed mechanistic studies highlighted a facile C-H cleavage with unique chemo-selectivity, while cyclovoltammetric analysis provided support for a nickel(II/III/IV) manifold.
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