Journal
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
Volume 58, Issue 6, Pages 1789-1793Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201811858
Keywords
carbonylation; photocatalysis; radicals; silicates; three-component reactions
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Funding
- JSPS [26248031, 17K05866]
- Scientific Research on Innovative Areas 2707: Middle Molecular Strategy from the MEXT [15H05850]
- Sorbonne University [ANR-17-CE07-0018 HyperSilight]
- Grants-in-Aid for Scientific Research [15H05850, 17K05866] Funding Source: KAKEN
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Primary, secondary, and tertiary alkyl radicals formed by the photocatalyzed oxidation of organosilicates underwent efficient carbonylation with carbon monoxide (CO) to give a variety of unsymmetrical ketones. This study introduces the possibility of radical carbonylation under a photooxidative regime.
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