Journal
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
Volume 58, Issue 7, Pages 2120-2124Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201811888
Keywords
enantioselective catalysis; fluorinated solvents; hydroformylation; phosphorus ligands; rhodium
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Funding
- Eastman Chemical Company
- EPSRC [EP/M003868/1]
- EPSRC [EP/M003868/1] Funding Source: UKRI
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The hydroformylation of propene to give predominantly iso-butanal has been achieved; class-leading selectivity is possible even at higher temperatures that deliver fast conversion. Racemic rhodium complexes of bidentate phospholane phosphites derived from tropos-biphenols and unusual solvent systems are the key to the selectivity observed.
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