Journal
ACS APPLIED MATERIALS & INTERFACES
Volume 10, Issue 44, Pages 38006-38014Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acsami.8b11672
Keywords
anode; carbon network; freestanding; SnO2 nanosheets; sodium-ion; batteries
Funding
- National Natural Science Foundation of China [51772337]
- Fund for Fostering Talents in State Key Laboratory of Optoelectronic Materials and Technologies, China [OEMT-2017-ZY-09]
- Fundamental Research Funds for the Central Universities, China [16lgjc60]
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Here, we demonstrate the in situ growth of SnO2 nanosheets on a freestanding carbonized eggshell membrane (CEM), which provides three-dimensional, bicontinuous electron and ion transport pathways through a massively interconnected carbon fiber skeleton and interpenetrated pore network, respectively. This CEM has other advantages such as the ability to alleviate mechanical stress during cycling as a buffer matrix. When used as an additive-free anode in a sodium-ion battery, SnO2 nanosheets can realize a complete electrochemical reaction and maintain good cycling stability with the help of a CEM. For instance, SnO2 nanosheets delivered a high reversible capacity of 656 mA h g(-1) in the 5th cycle at 0.1 A g(-1), approaching 98% of its theoretical specific capacity, and maintained a high reversible specific capacity of 420 mA h g(-1) after 200 cycles at 0.2 A g(-1).
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