Journal
SCIENCE ADVANCES
Volume 4, Issue 9, Pages -Publisher
AMER ASSOC ADVANCEMENT SCIENCE
DOI: 10.1126/sciadv.aau1698
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Funding
- Netherlands National Science Foundation (NWO)
- China Scholarship Council
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The development of new membranes with high H-2 separation performance under industrially relevant conditions (high temperatures and pressures) is of primary importance. For instance, these membranes may facilitate the implementation of energy-efficient precombustion CO2 capture or reduce energy intensity in other industrial processes such as ammonia synthesis. We report a facile synthetic protocol based on interfacial polymerization for the fabrication of supported benzimidazole-linked polymer membranes that display an unprecedented H-2/CO2 selectivity (up to 40) at 423 K together with high-pressure resistance and long-term stability (> 800 hours in the presence of water vapor).
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