Journal
APPLIED NANOSCIENCE
Volume 2, Issue 2, Pages 91-109Publisher
SPRINGER HEIDELBERG
DOI: 10.1007/s13204-011-0044-x
Keywords
Electrolytes; Lithium ion battery; Ionic liquids; Nanoparticle organic hybrids; Lithium/air; Lithium dendrites
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Funding
- King Abdullah University of Science and Technology (KAUST) [KUS-C1-018-02]
- National Science Foundation [DMR1006323]
- U.S. Department of Energy, Office of Basic Energy Sciences [DE-SC0001086]
- Materials for a Sustainable Future IGERT program, NSF [DGE-0903653]
- Division Of Materials Research
- Direct For Mathematical & Physical Scien [1006323] Funding Source: National Science Foundation
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From aqueous liquid electrolytes for lithium-air cells to ionic liquid electrolytes that permit continuous, high-rate cycling of secondary batteries comprising metallic lithium anodes, we show that many of the key impediments to progress in developing next-generation batteries with high specific energies can be overcome with cleaver designs of the electrolyte. When these designs are coupled with as cleverly engineered electrode configurations that control chemical interactions between the electrolyte and electrode or by simple additives-based schemes for manipulating physical contact between the electrolyte and electrode, we further show that rechargeable battery configurations can be facilely designed to achieve desirable safety, energy density and cycling performance.
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