4.7 Article

Preparation and adsorption capacity evaluation of graphene oxide-chitosan composite hydrogels

Journal

SCIENCE CHINA-MATERIALS
Volume 58, Issue 10, Pages 811-818

Publisher

SCIENCE PRESS
DOI: 10.1007/s40843-015-0090-x

Keywords

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Funding

  1. National Natural Science Foundation of China [21473153, 21207112]
  2. National Natural Science Foundation of Hebei Province [B2013203108]
  3. Science Foundation for the Excellent Youth Scholars from the Universities and Colleges of Hebei Province [YQ2013026]
  4. Support Program for the Top Young Talents of Hebei Province
  5. Scientific and Technological Research and Development Program of Qinhuangdao City [201502A006]
  6. Open Foundation of National Key Laboratory of Biochemical Engineering (Institute of Process Engineering, Chinese Academy of Sciences (CAS))

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Graphene oxide (GO)-chitosan composite hydrogels were successfully prepared via the self-assembly of chitosan molecules and GO. These as-prepared hydrogels were characterized by different techniques. The morphology of the internal network structure of the nanocomposite hydrogels was investigated. The adsorption capacity results demonstrate that the prepared GO-based composite hydrogels can efficiently remove three tested dye molecules, Congo red, methylene blue and Rhodamine B, from wastewater in accordance with the pseudo-second-order model. The dye adsorption capacity of the obtained hydrogels is mainly attributed to the GO sheets, whereas the chitosan molecule was incorporated to facilitate the gelation process of the GO sheets. The present study indicates that the as-prepared composite hydrogels can serve as good adsorbents for wastewater treatment as well as the removal of harmful dyes.

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