Journal
SCIENCE CHINA-MATERIALS
Volume 58, Issue 1, Pages 21-27Publisher
SCIENCE PRESS
DOI: 10.1007/s40843-014-0012-3
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Funding
- Ministry of Science and Technology of China [2011CB013000]
- National Natural Science Foundation of China [21325415, 21174019, 51161120361]
- Beijing Natural Science Foundation [2152028]
- Fok Ying Tong Education Foundation [131043]
- 111 Project [807012]
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Pt heterostructures can have distinctly different physical and chemical properties to their single-phase components. Herein, a smart approach was developed for the large-scale production of graphitic C3N4-Pt (gC(3)N(4)-Pt) heterostructures on three-dimensional (3D) graphene sheet networks for highly efficient methanol oxidation. Because the gC(3)N(4)-Pt heterostructures on the conductive 3D graphene network support provide the methanol molecules good accessibility to the active sites, the obtained catalyst exhibits excellent electrocatalytic performance, including high catalytic activity, unusual CO tolerance, and good stability, and is superior to commercial Pt/C and Pt/graphene catalysts for methanol oxidation.
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