Journal
ORGANIC CHEMISTRY FRONTIERS
Volume 5, Issue 19, Pages 2810-2814Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c8qo00734a
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Funding
- National Natural Science Foundation of China [21722203, 21702093, 21572096]
- Shenzhen special funds for the development of biomedicine, Internet, new energy, and new material industries [JCYJ20170412152435366, JCYJ20170307105638498]
- Shenzhen Nobel Prize Scientists Laboratory Project [C17213101]
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Diverse anti-Markovnikov hydrofunctionalization of alkenols triggered by the addition of S-, P-, and C-centered radicals to alkenes followed by intramolecular 1,5(6)-hydrogen atom transfer (HAT) with remote -C-H bonds of alcohols has been developed. The strategy simultaneously realized the hydrofunctionalization of alkenes and remote alcohol oxidation. This mild and versatile method allows for direct access to valuable sulfonyl-, phosphonyl-, and malonate-substituted ketones or aldehydes from a wide range of alkenols.
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