4.5 Article

Radiative Thermal Runaway Due to Negative-Differential Thermal Emission Across a Solid-Solid Phase Transition

Journal

PHYSICAL REVIEW APPLIED
Volume 10, Issue 2, Pages -

Publisher

AMER PHYSICAL SOC
DOI: 10.1103/PhysRevApplied.10.021001

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Funding

  1. Solid-State Solar Thermal Energy Conversion (S3TEC) Center, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-FG02-09ER46577]
  2. Office of Naval Research [N00014-16-1-2556, N00014-16-1-2398]

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Thermal runaway occurs when a rise in system temperature results in heat-generation rates exceeding dissipation rates. Here, we demonstrate that thermal runaway occurs in radiative (photon) systems given a sufficient level of negative-differential thermal emission. By exploiting the insulator-to-metal phase transition of vanadium dioxide, we show that a small increase in heat generation (e.g., 10 nW/mm(2)) results in a large change in surface temperature (e.g., similar to 35 K), as the thermal emitter switches from high emittance to low emittance. While thermal runaway is typically associated with catastrophic failure mechanisms, detailed understanding and control of this phenomenon may give rise to new opportunities in infrared sensing, camouflage, and rectification.

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