Journal
INORGANIC CHEMISTRY FRONTIERS
Volume 2, Issue 2, Pages 116-124Publisher
CHINESE CHEMICAL SOC
DOI: 10.1039/c4qi00115j
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- IIT Indore
- CSIR, New Delhi [01(2722)/13/EMR-II]
- SERB (DST), New Delhi
- UGC, New Delhi
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A highly active phosphine-free ruthenium-arene complex, [(eta(6)-C6H6)RuCl2(C6H5NH2)], exhibits excellent catalytic performance for a one-pot conversion of aldehydes to primary amides at low temperature (60 degrees C), in water and without any inert gas protection. The reported catalyst performed exceptionally well for a huge range of aldehydes, including aromatic, heteroaromatic, aliphatic and conjugated systems, with a high tolerance for other functional groups. The development of such highly active catalysts using simple reagents will offer new opportunities for the development of improved phosphine-free catalytic systems for this and other related catalytic reactions.
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