Journal
NANOSCALE RESEARCH LETTERS
Volume 7, Issue -, Pages -Publisher
SPRINGEROPEN
DOI: 10.1186/1556-276X-7-461
Keywords
redox reaction; metal-organic framework; CO oxidation; metal oxide; nanoparticle; palladium
Funding
- UNIST (Ulsan National Institute of Science and Technology)
- Basic Science Research Program through the National Research Foundation of Korea (NRF)
- Ministry of Education, Science and Technology [2011-0004358, 2012-0003813]
- POSCO TJ Park Foundation
- WCU (World Class University) [R-31-2008-10029]
- National Research Foundation of Korea [2010-0009063] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)
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The preparation of redox-active metal-organic framework (ra-MOF)-supported Pd nanoparticles (NPs) via the redox couple-driven method is reported, which can yield unprotected metallic NPs at room temperature within 10 min without the use of reducing agents. The Pd@ra-MOF has been exploited as a precursor of an active catalyst for CO oxidation. Under the CO oxidation reaction condition, Pd@ra-MOF is transformed into a PdOx-NiOy/C nanocomposite to generate catalytically active species in situ, and the resultant nanocatalyst shows sustainable activity through synergistic stabilization.
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