Journal
NANO ENERGY
Volume 53, Issue -, Pages 160-167Publisher
ELSEVIER
DOI: 10.1016/j.nanoen.2018.08.050
Keywords
Energy level; Interface contact; Oxygen management; Carbon electrode; Perovskite solar cell
Categories
Funding
- National Natural Science Foundation of China [91733301, 91433203, 61474049, 51502141, 21702069]
- Ministry of Science and Technology of China (863) [2015AA034601]
- Science and Technology Department of Hubei Province [2017AAA190]
- 111 Project [B07038]
- China Postdoctoral Science Foundation [2018M632844, 2016M602292]
- Science and Technology Department of Jiangsu Province [BK20150920]
- [2017T100548]
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Full-printable all-inorganic mesoporous network has emerged as a promising device scaffold for perovskite photovoltaic applications because of its highly stable device architecture and essentially scalable fabrication process, but practical application of this photovoltaic technology requires further advancement on power conversion efficiency. Here we introduce a facile oxygen management strategy in the carbon electrode (CE) to simultaneously tune energy alignment and the interface contact between perovskite and the CE. Augmenting the oxygen content of carbon black in CE not only elevates the energy level of the CE, but also optimizes the perovskite/CE interface contact, leading to a significantly enhanced hole extraction efficiency at the interface of perovskite/CE. These enable us to fabricate solar cells possessing a maximum efficiency of 15.7% benefiting from open-circuit voltage enhancement of 100 mV, which is significantly higher than that of control device (13.6%) without oxygen management in the CE. The present work diversifies a strategy to optimize the energy level alignment and interface contact of the perovskite/CE for the efficient printable mesoscopic perovskite solar cells.
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