Journal
JOURNAL OF MATERIALS CHEMISTRY A
Volume 6, Issue 41, Pages 20138-20144Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c8ta07617k
Keywords
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Funding
- National Research Foundation of Korea grant (NRF) [2016R1C1B2016188, 2017R1A2B3010049]
- Development Program of the Korea Institute of Energy Research (KIER) [B8-2421, B8-2425]
- U-K Brand of Ulsan National Institute of Science and Technology (UNIST) [1.180043.01]
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Processing for obtaining compact and uniform perovskite photoactive layers has been intensively studied over the last few years to achieve high power conversion efficiencies (PCEs) in solar cells. Particularly, high quality crystal growth of perovskite layers is critical to enhance device performance. We demonstrate an easy and effective new process for high efficiency p-i-n planar heterojunction structures of perovskite solar cells (PeSCs) by using a compact seed perovskite layer (CSPL). The CSPL assists vertical growth of perovskite crystals and obtains the highly crystalline perovskite photoactive layer, which leads to the reduction in the charge transfer resistance and a longer photoluminescence lifetime. The PeSC device with a CSPL shows a remarkably improved PCE, from 15.07% to 19.25%, with a record open circuit voltage (V-OC) of 1.16 V in the p-i-n structure with pure crystal perovskite and negligible current density-voltage hysteresis. Additionally, a PCE of 20.37% was achieved in CSPL assisted n-i-p structure PeSCs.
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