Journal
JOURNAL OF MATERIALS CHEMISTRY A
Volume 6, Issue 41, Pages 20365-20373Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c8ta06719h
Keywords
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Funding
- National Natural Science Foundation of China [21403112]
- Fundamental Research Funds for the Central Universities [3091501333]
- Priority Academic Program Development of Jiangsu Higher Education Institutions (PAPD)
- Postgraduate Research AMP
- Practice Innovation Program of Jiangsu Province
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All-inorganic perovskite cesium lead triiodine (CsPbI3) is emerging as a promising thermally stable light absorber in flexible optoelectronic devices. However, the photoactive alpha-CsPbI3 only exists at a temperature higher than 310 degrees C and rapidly degrades to the undesired delta-CsPbI3 at room temperature. Here, a vacuum-assisted drying process is first developed to fabricate all-inorganic perovskite thin films at room temperature. The film morphology and photoelectric properties as well as the long-time stability are significantly improved compared to those of the reference film fabricated with annealing process. The flexible solar cells based on such room temperature processed films demonstrate a high power conversion efficiency of 11.47% with a small hysteresis. Moreover, the champion flexible cell also exhibits high air-stability and excellent flexibility. These results offer a new pathway for developing high-performance and cost-effective flexible optoelectronic devices.
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