Journal
JOURNAL OF MATERIALS CHEMISTRY A
Volume 2, Issue 18, Pages 6598-6604Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c3ta15110g
Keywords
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Funding
- National Science Foundation of China [11174103, 90923032]
- Specialized Research Fund for the Doctoral Program of Higher Education of China [20130061110012]
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Nanoscale Ag-loaded sunflower-like In2O3 hierarchical nanostructures are developed for HCHO detection. Such unique architectures are synthesized by an ambient temperature and pressure hydrolysis reaction combined with a subsequent chemical reduction process. Morphology characterizations confirm that homodisperse nanochains assembled by nanoparticles along the same direction are radially linked to a center to construct sunflower-like hierarchical nanostructures. Novel highly porous and branched structure of the 3D hierarchical architectures and the chemical and electronic sensitization effect of Ag nanoparticles endow Ag-loaded In2O3 nanostructures-based sensors with enhanced gas sensing performances in terms of fast response time (0.9 s), recovery time (14 s), high sensitivity and good sensing selectivity for 20 ppm HCHO. A multistage reaction formation mechanism of the sunflower-like hierarchical nanostructures, and a morphology-dependent sensing mechanism are proposed.
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