4.6 Article

Engineering crystalline structures of two-dimensional MoS2 sheets for high-performance organic solar cells

Journal

JOURNAL OF MATERIALS CHEMISTRY A
Volume 2, Issue 21, Pages 7727-7733

Publisher

ROYAL SOC CHEMISTRY
DOI: 10.1039/c4ta01336k

Keywords

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Funding

  1. National Basic Research Program [2014CB643503, 2014CB932500]
  2. National Natural Science Foundation of China [91233114, 51261130582, 50990063, 51222202]
  3. Zhejiang Provincial Natural Science Foundation of China [R4110030]
  4. Science and Technology Department of Zhejiang Province [2011R10077]
  5. Program for New Century Excellent Talents in University [NCET-12-0494]
  6. Research Fund for the Doctoral Program of Higher Education [20130101110123]
  7. Program for 14th China-Japan ST Cooperation [2013DFG52800]
  8. Program for Innovative Research Team in the University of Ministry of Education of China [IRT13037]

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The effects of different local crystalline structures on two-dimensional (2D) MoS2 sheets are studied to provide new insights into how the local characteristics affect the performance of organic solar cells (OSCs) and how to tailor the local characteristics towards high-performance devices. UV-ozone post-treatment of 2D MoS2 sheets led to incorporation of oxygen atoms into the lattice of the sheets. The incorporated oxygen in 2D MoS2 sheets significantly improved the performance of OSCs, where 2D MoS2 sheets were used as hole transport layers.

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