Journal
JOURNAL OF MATERIALS CHEMISTRY A
Volume 2, Issue 36, Pages 14827-14834Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c4ta01749h
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Funding
- NSFC of China [21001022, 21171033, 21131001, 21222105, 20801041]
- PhD Station Foundation of Ministry of Education [20100043110003]
- Foundation for Author of National Excellent Doctoral Dissertation of P.R.China (FANEDD) [201022]
- Science and Technology Development Planning of Jilin Province [20111803]
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Five isostructural pillared-layer MOFs (metal-organic frameworks) have been constructed by selection of layers and size-alterable pillar ligands. These MOFs show similar structures but different interlayer distances, pore volumes and pore surface functionalizations depending on the lengths and functions of pillar ligands. 1-5 display a certain degree of framework stabilities, and also exhibit CO2 uptakes. In addition, 1 can serve as a host for encapsulating I-2 and exhibit an outstanding performance in reversible adsorption of iodine molecules. Furthermore, 1-5 can be used to separate dye molecules based on the size-exclusion effect and 3 can be employed as a column-chromatographic filler to separate Rhodamine B (RB) and Methylene Blue (MB).
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