Journal
JOURNAL OF MATERIALS CHEMISTRY A
Volume 2, Issue 13, Pages 4514-4519Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c3ta14783e
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Funding
- CSIR, New Delhi
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A chemically functionalized nanocrystalline TiO2 grafted ruthenium(II) polyazine complex was found to be an efficient visible light photoredox catalyst for the oxidative cyanation of tertiary amines to the corresponding alpha-aminonitriles in high to excellent yields, using molecular oxygen as an oxidant and sodiumcyanide in acetic acid as a cyanide source. The developed photoredox catalyst could be easily recovered by simple filtration and reused for several runs with consistent catalytic activity.
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