Journal
JOURNAL OF MATERIALS CHEMISTRY A
Volume 2, Issue 7, Pages 2168-2173Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c3ta14267a
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Funding
- 973 Program [2013CB834704]
- National Natural Science Foundation of China [21231002, 21173021, 21276026, 21201018]
- 111 Project [B07012]
- Program of Co-operation of the Beijing Education Commission [20091739006]
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We report a strategy to synthesize materials in which POMs are enclosed in the cages of ZIFs. In three new compounds, H3PW12O40 subset of ZIF-8 (BIT-1), H4SiW12O40 subset of ZIF-8 (BIT-2) and H3PMo12O40 subset of ZIF-8 (BIT-3), different POM cages are 'trapped' inside the well-defined cages of ZIF-8 by one-pot mechanochemical synthesis. They show the highest capacity for methylene blue and controlled release of the anti-cancer agent 5-fluorouracil. BITs can be fully recovered and reused without losing their uptake capacity.
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