Journal
JOURNAL OF MATERIALS CHEMISTRY A
Volume 1, Issue 7, Pages 2543-2551Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c2ta01260j
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Funding
- Welch Foundation [AX-1730]
- DOE BES [DE-FG02-08ER46522]
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A NbO-type metal-organic framework UTSA-40 constructed from a novel aromatic tetracarboxylate has been synthesized and structurally characterized. With open metal sites, suitable pore spaces and a moderate BET surface area of 1630 m(2) g(-1) for the recognition of CO2 and CH4, the activated UTSA-40a has the potential for use in H-2 purification processes conducted in fixed bed adsorbers, with higher productivities and lower regeneration costs than those obtained with conventionally used NaX and LTA-5A zeolites when operating at higher pressure. Furthermore, its regeneration cost is also lower than that of the examined MOFs MgMOF-74 and Cu-TDPAT despite its lower productivity.
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