Journal
JOURNAL OF MATERIALS CHEMISTRY A
Volume 1, Issue 3, Pages 752-758Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c2ta00616b
Keywords
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Funding
- National Basic Research Program of China (973 Program) [2012CB821700]
- NSFC [21120102034, 20831002]
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Novel porous aromatic frameworks, PAF-18-OH and its lithiated derivative PAF-18-OLi, have been successfully synthesized. In particular, PAF-18-OLi displays significant enhancement of H-2 and CO2 adsorption capacity, especially for CO2 uptake (14.4 wt%). More valuably, the stable PAF-18-OLi material exhibits high CO2/N-2 selectivity, as high as 129 in the case of CO2 capture from simulated post-combustion flue gas mixtures (85% N-2 and 15% CO2). Furthermore, the PAF-18-OLi has shown improved H-2 storage capacity after lithiation.
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