Journal
JOURNAL OF MATERIALS CHEMISTRY A
Volume 1, Issue 26, Pages 7775-7781Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c3ta10457e
Keywords
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Funding
- U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-SC0005397]
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Holey graphene (HG) synthesized by a hydrothermal method followed by etching with KOH and ball milling is randomly stacked to form a porous structure. These randomly stacked holey graphene anodes exhibit high rate capability with excellent cycling stability as an anode material for lithium-ion cells. This fascinating electrochemical performance can be ascribed to their specific porous structure, providing numerous active sites for Li+ insertion, reduced effective diffusion distance for the Li+ ions, high electrical conductivity, low charge-transfer resistance across the electrolyte-electrode interface, and improved structural stability against the local volume change during Li+ insertion-extraction.
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