Journal
JOURNAL OF MATERIALS CHEMISTRY A
Volume 1, Issue 46, Pages 14658-14665Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c3ta13370b
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Funding
- Fundamental Research Funds for the Central Universities [FRF-SD-12-007A]
- National Natural Science Foundation of China [21276023]
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We demonstrate the fabrication of three-dimensional nitrogen-doped graphene (3D N-G)/nanoparticle anode architectures consisting of 3D N-G networks and Fe3O4 nanoparticles. In such a hybrid structure, the N-G networks act as a buffer matrix to accommodate the volume change of Fe3O4, and the interconnected N-G sheets effectively prevent the aggregation of nanoparticles during cycling, both of which enable the structural integrity and electrochemical stabilization of such composite electrodes. Furthermore, the as-obtained porous nitrogen-doped hybrid materials promote efficient transport of both lithium ions and electrons upon charging/discharging, and also provide defect sites as Li+ active sites on the surface of N-G sheets. As a result, the hybrids exhibit much-improved lithium storage performance.
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