Journal
ADVANCED OPTICAL MATERIALS
Volume 1, Issue 11, Pages 827-833Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adom.201300256
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Funding
- UK Engineering and Physical Sciences Research Council via the Active Plasmonics programme grant [EP/H000917/1]
- Engineering and Physical Sciences Research Council [EP/H000917/2, EP/D063329/1, EP/H000917/1] Funding Source: researchfish
- EPSRC [EP/D063329/1, EP/H000917/2, EP/H000917/1] Funding Source: UKRI
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Ultrastrong exciton-photon coupling of Frenkel molecular excitons is demonstrated at room temperature in a metal-clad microcavity containing a thin film of 2,7-bis[9,9-di( 4-methylphenyl)-fluoren-2-yl]-9,9-di( 4- methylphenyl) fluorene. A giant Rabi splitting of Omega 1 eV is measured using angle-resolved reflectivity and bright photoluminescence is observed from the lower polariton branch. To obtain the virtual photon and exciton content of the polariton ground state, the results are interpreted in terms of the full Hopfield Hamiltonian, including anti-resonant terms. Also included is an analytical treatment of the often ignored and sometimes misinterpreted TM-polarized metal-insulatormetal plasmon-polariton.
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