Journal
ACS MACRO LETTERS
Volume 1, Issue 11, Pages 1300-1303Publisher
AMER CHEMICAL SOC
DOI: 10.1021/mz300456p
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Funding
- National Natural Science Foundation of China [21090351]
- 973 Project [2011CB201402]
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Multicomponent polymerization based on Passerini reaction is described. Room temperature polymerization of dicarboxyl acid, monoaldehyde, and diisocyanide leads to the formation of a new type of sequence regulated poly(ester-amide)s in an efficient one-pot process. The polymerization was confirmed to be a stepwise mechanism, and the resulting polymers were characterized and determined to be linear polymers with a sequence regulated backbone repeating unit of esteresteramideamide. When functional aldehydes were used, functional side groups could be easily introduced at the same time, providing a simple way for further modification.
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