Journal
SCIENTIFIC REPORTS
Volume 5, Issue -, Pages -Publisher
NATURE PUBLISHING GROUP
DOI: 10.1038/srep14414
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Funding
- CREST of JST
- JSPS [15H05697]
- APSA from MEXT
- DOWA Technofund
- MEXT
- Grants-in-Aid for Scientific Research [26810045, 26708008, 15H05697] Funding Source: KAKEN
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Development of nanometer-sized magnetic particles exhibiting a large coercive field (H-c) is in high demand for densification of magnetic recording. Herein, we report a single-nanosize (i.e., less than ten nanometers across) hard magnetic ferrite. This magnetic ferrite is composed of epsilon-Fe2O3, with a sufficiently high H-c value for magnetic recording systems and a remarkably high magnetic anisotropy constant of 7.7 x 10(6) erg cm(-3). For example, 8.2-nm nanoparticles have an H-c value of 5.2 kOe at room temperature. A colloidal solution of these nanoparticles possesses a light orange color due to a wide band gap of 2.9 eV (430 nm), indicating a possibility of transparent magnetic pigments. Additionally, we have observed magnetization-induced second harmonic generation (MSHG). The nonlinear optical-magnetoelectric effect of the present polar magnetic nanocrystal was quite strong. These findings have been demonstrated in a simple iron oxide, which is highly significant from the viewpoints of economic cost and mass production.
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