Journal
ADVANCED MATERIALS INTERFACES
Volume 2, Issue 14, Pages -Publisher
WILEY
DOI: 10.1002/admi.201500220
Keywords
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Funding
- Natural Science Foundation of Jiangsu Province of China [BK20130313, BK20140400]
- National Natural Science Foundation of China [91027039, 51373110, 51203108, 51273134]
- Deanship of Scientific Research at King Saud University [PRG-1436-03]
- Priority Academic Program Development of Jiangsu Higher Education Institutions (PAPD)
- Qing Lan Project for Excellent Scientific and Technological Innovation Team of Jiangsu Province
- Project for Jiangsu Scientific and Technological Innovation Team
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Inspired by the hierarchical structure of the mastoid on the micrometer and nanometer scale and the waxy crystals of the mastoid on natural lotus surfaces, a facile one-step hydrothermal strategy is developed to coat flower-like hierarchical TiO2 micro/nanoparticles onto cotton fabric substrates (TiO2@Cotton). Furthermore, robust superhydrophobic TiO2@Cotton surfaces are constructed by the combination of hierarchical structure creation and low surface energy material modification, which allows versatility for self-cleaning, laundering durability, and oil/water separation. Compared with hydrophobic cotton fabric, the TiO2@Cotton exhibits a superior antiwetting and self-cleaning property with a contact angle (CA) lager than 160 degrees and a sliding angle lower than 5 degrees. The superhydrophobic TiO2@Cotton shows excellent laundering durability against mechanical abrasion without an apparent reduction of the water contact angle. Moreover, the micro/nanoscale hierarchical structured cotton fabrics with special wettability are demonstrated to selectively collect oil from oil/water mixtures efficiently under various conditions (e.g., floating oil layer or underwater oil droplet or even oil/water mixtures). In addition, it is expected that this facile strategy can be widely used to construct multifunctional fabrics with excellent self-cleaning, laundering durability, and oil/water separation. The work would also be helpful to design and develop new underwater superoleophobic/superoleophilic materials and microfluidic management devices.
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