Journal
ADVANCED MATERIALS INTERFACES
Volume 2, Issue 12, Pages -Publisher
WILEY
DOI: 10.1002/admi.201500163
Keywords
FeS2-sensitized ZnO@ZnS nanorods; heterostructures; optical absorption; photoresponse; ZnO@ZnS nanorods
Funding
- National Science Foundation of China [21301155]
- Zhejiang Provincial Natural Science Foundation of China [LR14B060002]
- National High Technology Research and Development Program (863) of China [2011AA11A101]
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FeS2-sensitized ZnO@ZnS nanorod arrays are fabricated by a two-step solution immersion and a subsequent sulfurization. The material properties including structure, morphology, and photoluminescence are investigated by a variety of characterization methods. As compared with ZnO@ZnS core/shell structure, FeS2-sensitized ZnO@ZnS nanorod arrays show improved optical absorption property with the extension of the absorption edge into the range of visible light. The photoresponse performance of FeS2-sensitized Zno@ZnS is also enhanced as the photocurrent density at 1.0 V is dozens of times larger than that of ZnO@ZnS nanorods. The cause for the difference in such material properties of these two materials is discussed. In this work, a new method for sensitizing wide bandgap ZnO@ZnS nanorod arrays with improved light response performance is presented.
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