4.6 Article

Nonlinear Interference and Tailorable Third-Harmonic Generation from Dielectric Oligomers

Journal

ACS PHOTONICS
Volume 2, Issue 5, Pages 578-582

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acsphotonics.5b00065

Keywords

nonlinear optics; third-harmonic generation; silicon nanoparticles; nanoparticle oligomers; optical magnetism; Mie scattering

Funding

  1. Russian Science Foundation [14-12-01144]
  2. Russian Foundation for Basic Research
  3. Australian Research Council
  4. U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]
  5. Russian Science Foundation [14-12-01144] Funding Source: Russian Science Foundation

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It is known that the nonlinear optical properties of photonic nanostructures can be modified substantially due to strong field confinement and optical resonances. In this contribution, we study third-harmonic generation from low-loss subwavelength silicon nanodisks arranged in the form of trimer oligomers with varying distance between the nano-particles. Each of the nanodisks exhibits both electric and magnetic Mie-type resonances that are shown to affect significantly the nonlinear response. We observe the third-harmonic radiation intensity that is comparable to that of a bulk silicon slab and demonstrate a pronounced reshaping of the third-harmonic spectra due to interference of the nonlinearly generated waves augmented by an interplay between the electric and the magnetic dipolar resonances.

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